I'm not positive, but I doubt it very much.
If you're talking about a bog standard calculator, I'm fairly certain it can't be done. There may be more scope with scientific calculators, but there are few problems that occur to me.
For example, would you include 0 in the numbers generated, how many sets of numbers do you want, how many digits are there to be in each series of numbers and what is the maximum range of numbers.
I don't think even programmable calculators are up to this task.
Why don't you try something like this?
http://www.randomizer.org/form.htm