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The British Empire is by far the largest in history? at least 60% larger than the next largest, the Mongol Empire. At one time covering approx 27% of the world. OK 5C, you're up.....
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For more on marking an answer as the "Best Answer", please visit our FAQ.According to Guinness World Records, in terms of the world's population at the time, it wasn't the largest empire as a percentage of that population.
"By share of population, the largest empire was the Achaemenid Empire, better known as the Persian Empire, which accounted for approximately 49.4 million of the world’s 112.4 million people in around 480 BC – an astonishing 44%. Originating in modern-day Iran, the empire was first established by Cyrus the Great and included parts of Central Asia, the Mediterranean, North Africa, and even European territories such as ancient Thrace and Macedonia."
"By share of population, the largest empire was the Achaemenid Empire, better known as the Persian Empire, which accounted for approximately 49.4 million of the world’s 112.4 million people in around 480 BC – an astonishing 44%. Originating in modern-day Iran, the empire was first established by Cyrus the Great and included parts of Central Asia, the Mediterranean, North Africa, and even European territories such as ancient Thrace and Macedonia."